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Winison is a Windows GUI front-end to Unison, the greatest synchronization program ever. Winison can manage profiles, generate the annoyingly-complicated windows batch files that simplify life, and also create windows "Send To" links enabling you to synchronize individual files or folders from within Windows. It's main purpose is to remove the need for you to learn Windows batch scripting (icky) or dig through your system to find your ".unison" and "Send To" folders. You will still need to learn how to use Unison however :).

Features:

Create, edit, save, load, delete, and/or run Unison profiles from a centralized interface.
Right-click a sub-folder and send it to Unison for synchronizing (awesome).
All of the sweet synchronizing features included with Unison, such as two-way synchronization of file changes (i.e. delta sync) and backing up older versions of overwritten files.